Dienone Explained

Dibenzylideneacetone is a well known dienone|thumb|right|240px

A dienone is a class of organic compounds with the general formula, where R is any substituent, but often H. They are formally "derived from 1,4-diene compounds by conversion of a –CH2– group into –C(=O)– group", resulting in "a conjugated structure". They are a kind of enone. The class includes some heterocyclic compounds.

Properties and occurrence

There is no evidence that phenols tautomerizes to a dienone, but such tautomerism is well recognized for resorcinols and some hydroxypyridines.

Being multifunctional, dienones engage in many reactions. They are often good dienophiles. They function as ligands, forming metal-alkene complexes such as tris(dibenzylideneacetone)dipalladium(0).

Cyclic dienones

Extensive work has been reported on cyclic dienones. The parent of the seven-membered ring series is tropone. It is a not only a dienone but a trieneone.

Cyclohexadienones are a significant class of dienones, the premier members being the ortho- and para-quinones. Many cyclohexadienones convert to phenols.[1] In the dienone–phenol rearrangement, they convert to phenols[2] through the dienone–phenol rearrangement:[3]

The parent cyclopentadienone has only a fleeting existence under laboratory conditions, otherwise it dimerizes. The substituted derivative tetraphenylcyclopentadienone is however robust solid.[4]

See also

Notes and References

  1. 10.1021/cr9803838 . Nucleophilic Additions to 4,4-Disubstituted 2,5-Cyclohexadienones: Can Dipole Effects Control Facial Selectivity? . 1999 . Wipf . Peter . Jung . Jae-Kyu . Chemical Reviews . 99 . 5 . 1469–1480 . 11749453 .
  2. Related to quinones, see for example the Zincke-Suhl reaction
  3. Advanced organic Chemistry, Reactions, mechanisms and structure 3ed. page Jerry March
  4. 10.1021/cr60235a001 . Chemistry of Cyclopentadienones . 1965 . Ogliaruso . Michael A. . Romanelli . Michael G. . Becker . Ernest I. . Chemical Reviews . 65 . 3 . 261–367 .