Α-Tocopherol Explained

α-Tocopherol (alpha-tocopherol) is a type of vitamin E. Its E number is "E307". Vitamin E exists in eight different forms, four tocopherols and four tocotrienols. All feature a chromane ring, with a hydroxyl group that can donate a hydrogen atom to reduce free radicals and a hydrophobic side chain, along with an aromatic ring is situated near the carbonyls in the fatty acyl chains of the phospholipid bilayer, allows for penetration into biological membranes.[1] It is found most in the membrane's non-raft domains, associated with omega-3 and 6 fatty acids, to partially prevent oxidation.[2] The most prevalent form, α-tocopherol, is involved in molecular, cellular, biochemical processes closely related to overall lipoprotein and lipid homeostasis. Compared to the others, α-tocopherol is preferentially absorbed and accumulated in humans.

Vitamin E is found in a variety of tissues, being lipid-soluble, and taken up by the body in a wide variety of ways. Ongoing research is believed to be "critical for manipulation of vitamin E homeostasis in a variety of oxidative stress-related disease conditions in humans."[3] One of these disease conditions is the α-tocopherol role in the use by malaria parasites to protect themselves from the highly oxidative environment in erythrocytes.[4] A second of these disease conditions is the α-tocopherol antioxidant properties' role cardiovascular heart disease. In preventing LDL (low-density lipoprotein) oxidation, it is able to decrease chances of atherosclerosis and arterial build-up.[5]

Synthesis

To synthesize the ⍺-diastereomer selectively, tocol acetate is transformed to the naturally occurring, kinetically favored α-Tocopherol after being catalyzed by the lipase enzyme. This reaction occurs under biological conditions, commonly in the digestive system.[6]

Stereoisomers

α-Tocopherol has three stereocenters, so it is a chiral molecule.[7] The eight stereoisomers of α-tocopherol differ in the configuration of these stereocenters. RRR-α-tocopherol is the natural one.[8] The older name of RRR-α-tocopherol is d-α-tocopherol, but this d/l naming should no longer be used, because whether l-α-tocopherol should mean SSS enantiomer or the SRR diastereomer is not clear, from historical reasons. The SRR may be named 2-epi-α-tocopherol, the diastereomeric mixture of RRR-α-tocopherol and 2-epi-α-tocopherol may be called 2-ambo-α-tocopherol (formerly named dl-α-tocopherol). The mixture of all eight diastereomers is called all-rac-α-tocopherol.[9] The α-Tocopherol is the most active diastereomer biologically, while being maintained at a high level in plasma and tissues of many different animal species.[10]

One IU of tocopherol is defined as milligram of RRR-α-tocopherol (formerly named d-α-tocopherol). 1 IU is also defined as 0.9 mg of an equal mix of the eight stereoisomers, which is a racemic mixture, all-rac-α-tocopheryl acetate. This mix of stereoisomers is often called dl-α-tocopheryl acetate.[11] Starting with May 2016, the IU unit is made obsolete, such that 1 mg of "Vitamin E" is 1 mg of d-alpha-tocopherol or 2 mg of dl-alpha-tocopherol.[12]

Notes and References

  1. Burton . G. W. . Ingold . K. U. . Vitamin E: application of the principles of physical organic chemistry to the exploration of its structure and function . Accounts of Chemical Research . 1 June 1986 . 19 . 7 . 194–201 . 10.1021/ar00127a001.
  2. Atkinson . Jeffrey . Harroun . Thad . Wassall . Stephen R. . Stillwell . William . Katsaras . John . The location and behavior of α‐tocopherol in membranes . Molecular Nutrition & Food Research . May 2010 . 54 . 5 . 641–651 . 10.1002/mnfr.200900439.
  3. Rigotti A . Absorption, transport, and tissue delivery of vitamin E . Molecular Aspects of Medicine . 28 . 5–6 . 423–36 . 2007 . 17320165 . 10.1016/j.mam.2007.01.002 .
  4. Shichiri M, Ishida N, Hagihara Y, Yoshida Y, Kume A, Suzuki H . Probucol induces the generation of lipid peroxidation products in erythrocytes and plasma of male cynomolgus macaques . Journal of Clinical Biochemistry and Nutrition . 64 . 2 . 129–142. 2019 . 30936625 . 6436040 . 10.3164/jcbn.18-7.
  5. Singh . U. . Devaraj . S. . Jialal . I. . VITAMIN E, OXIDATIVE STRESS, AND INFLAMMATION . Annual Review of Nutrition . 21 August 2005 . 25 . 1 . 151–174 . 10.1146/annurev.nutr.24.012003.132446.
  6. Mizuguchi . Eisaku . Takemoto . Masumi . Achiwa . Kazuo . An enzyme-catalyzed synthesis of natural α-tocopherol . Tetrahedron: Asymmetry . January 1993 . 4 . 9 . 1961–1964 . 10.1016/s0957-4166(00)82239-9.
  7. Jensen SK, Lauridsen C . Alpha-tocopherol stereoisomers . Vitamins and Hormones . 76 . 281–308 . 2007 . 17628178 . 10.1016/S0083-6729(07)76010-7 . 9780123735928 .
  8. Brigelius-Flohé R, Traber MG . Vitamin E: function and metabolism . FASEB Journal . 13 . 10 . 1145–55 . July 1999 . 10385606 . 10.1096/fasebj.13.10.1145 . 7031925 . free .
  9. https://web.archive.org/web/20201122071533/https://www.qmul.ac.uk/sbcs/iupac/misc/toc.html IUPAC Nomenclature of Tocopherols and Related Compounds
  10. Jensen . Søren K. . Nørgaard . Jan V. . Lauridsen . Charlotte . Bioavailability of α-tocopherol stereoisomers in rats depends on dietary doses of all-rac - or RRR-α-tocopheryl acetate . British Journal of Nutrition . March 2006 . 95 . 3 . 477–487 . 10.1079/bjn20051667 . 31 October 2024.
  11. Web site: https://web.archive.org/web/20120219164132/http://www.nal.usda.gov/fnic/foodcomp/Data/SR20/SR20_doc.pdf . 2012-02-19 . Composition of Foods Raw, Processed, Prepared USDA National Nutrient Database for Standard Reference, Release 20 . . February 2008 . dead .
  12. Web site: Unit Conversions . . 2018-11-21.